All of the mark 4s involved in Great Heck were written off and scrapped, as well as some of those involved in the Hatfield accident. Although those that were appeared to be in a much poorer structural condition than the carriages of 390033 at Grayrigg from a cursory glance. I mean, DVT 82221 that was involved in the Great Heck crash was entirely demolished, and the restaurant vehicle that went into the catenary mast at Hatfield (10327) was in no great shape either.
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Is there anything stopping them being used to extend some of the 9-car Pendolinos? Presumably this idea has been put forward before.
As other posters have said, it was cheaper to withdraw the unit as an insurance write-off than to return certain vehicles out of the set to passenger service.
Plus, it's not as simple as just inserting any old vehicles into the Pendolinos to extend them. Of the two additional vehicles being inserted into the Pendolinos to make them into 11 carriage formations, one is a trailer standard and the other a motor standard. The motor standard will become the centre vehicle in the train and carries a third transformer and other electrical gubbins that the other motor vehicles do not have. Additionally, a Pendolino in 9 carriage formation has three trailer vehicles; one the additional ninth vehicle in the centre of the formation, and the other two the pantograph cars. The central trailer vehicle of 390033 (68833) was one of the carriages that didn't survive, and I suspect that the two pantograph cars, 69533 and 69833 which are still extant, would probably need some sort of system reboot or rewire (plus the transformers and pantograph removing) to make them compatible as basic trailers.