Dartford should be part of Greater London (as should Epsom, Staines, Watford etc.), if it was, it'd probably be a GLA strategic opportunity area for redevelopment and Liz Line would key for it - Dartford is only as far out as Romford/Hornchurch. No politician is brave enough to support the expansion of Gtr. London further, but I digress...
Expensive option:
Dartford should certainly have fast trains and is a victim of not being on a main line. If we were to extend Crossrail to Dartford or Gravesend, I think the 4 tracks should be in place and perhaps controversially, Crossrail should run fast to Dartford, with Thameslink scrapped and all Southeastern Dartford lines back at 4-8tph. Crossrail then extends to Gravesend on the current tracks, shared with 4tph Southeastern (2tph each Bexleyheath & Sidcup).
If it helps SE capacity and punctuality, I would consider scrapping rounders, making Dartford a *Zone 6* interchange hub, and rebuilding Dartford station with enough platforms to do so (have a local regen project as part of it). Then, **real crayonista** extend the Goblin from Barking Riverside to Thamesmead, Abbey Wood and Bexleyheath to silence a lack of SE connectivity concerns.
In the West I would, rather than the large expensive Southern access project that'll happen once millennials are long buried, extend Crossrail from Heathrow 5 to Staines. Wouldn't cost peanuts, but it'd certainly be worthwhile. So if you could get more Liz Line on the GWML, I would send them there.
But considering OOC is coming, Royal Kensington & TfL want a station at Kensal Canalside, and City Airport also wants (should have) a station, how much can we really have without train lengthening and doing what Île-de-France is doing by needing RER E??